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Photoactive Metal-Organic Framework for Solar-Driven Atmospheric Water Harvestin...

Photoactive Metal-Organic Framework for Solar-Driven Atmospheric Water Harvesting in Arid Climates Atmospheric water harvesting (AWH) using solar energy has gained significant attention; however, its application in arid climates poses challenges due to low relative humidity (RH) and reduced efficiency of conventional sorbents.... ver más

31/10/2026

UCM

181K€

Presupuesto del proyecto: 181K€

Líder del proyecto

Universidad Complutense de Madrid No se ha especificado una descripción o un objeto social para esta compañía.

Total investigadores 3281

Fecha límite participación Sin fecha límite de participación.

Financiación concedida El organismo HORIZON EUROPE notifico la concesión del proyecto el día 2024-03-13

HORIZON-MSCA-2023-PF-01-01: MSCA Postdoctoral Fellowships 2023 ExpectedOutcome:Project results are expected to contribute to the following outcomes:

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1 Participantes

UCM

181.15K€ | Lider

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Duración del proyecto: 31 meses Fecha Inicio: 2024-03-13
Fecha Fin: 2026-10-31

Líder del proyecto

Universidad Complutense de Madrid No se ha especificado una descripción o un objeto social para esta compañía.

Total investigadores 3281

Presupuesto del proyecto 181K€

Fecha límite de participación Sin fecha límite de participación.

Descripción del proyecto Atmospheric water harvesting (AWH) using solar energy has gained significant attention; however, its application in arid climates poses challenges due to low relative humidity (RH) and reduced efficiency of conventional sorbents. metal-organic frameworks (MOFs) are a class of porous materials with an engineerable structure that have the ability to capture water even at very low RH. Usually, the combination of photothermal materials with MOFs is used to desorb water sorbed by MOFs. One of the challenges of this method is the reduction of MOF sorption capacity, which is very unfavorable, especially in arid climates. Reducing the performance of sorbents in arid climates due to the blocking of sorption sites by dust is another challenge that has received little attention so far. To address these challenges, this study evaluates the synthesis of a unique water-stable MOF with photothermal and photocatalytic (photoactive) properties (PAMOF), in addition to high water affinity. Phthalocyanine and porphyrin ligands decorated with Ti and Cu ions, along with Yttrium (Y) and Erbium (Er) clusters, are considered as promising candidates. Molecular modeling using density functional theory (DFT) will be conducted to guide the synthesis process, followed by experimental synthesis and characterization. Subsequently, the samples will be evaluated in an AWH device to assess short-term efficiency and long-term maintenance in real conditions. In addition to harnessing natural solar energy, the AWH experiments will involve the utilization of a custom-made solar simulator. The SAWH device will be evaluated across a range of RHs, spanning from 10% to 90%, while considering the presence of artificial dust. Through comparative analysis of existing research and with the aim of enhancing previously studied systems, this project endeavors to attain a daily water evaporation rate surpassing 4 kgwater/kgPAMOF under 1 sun and RH<30.

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