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Photo ElectroCatalysis New activation paradigm

Due to a high sustainability and to a straightforward tunability of the energy input (wavelength, redox potential), the use of light and electricity for the activation of organic molecules constitutes an attractive method in the t... ver más

30/04/2022

UK BA

143K€

Presupuesto del proyecto: 143K€

Líder del proyecto

UNIVERZITA KOMENSKEHO V BRATISLAVE No se ha especificado una descripción o un objeto social para esta compañía.

TRL 4-5

Fecha límite participación Sin fecha límite de participación.

Financiación concedida El organismo H2020 notifico la concesión del proyecto el día 2022-04-30

MSCA-IF-2019: Individual Fellowships

I+D

Cerrada hace 5 años

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Información adicional privada

No hay información privada compartida para este proyecto. Habla con el coordinador.

1 Participantes

UK BA

143.36K€ | Lider

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Duración del proyecto: 25 meses Fecha Inicio: 2020-03-28
Fecha Fin: 2022-04-30

Líder del proyecto

UNIVERZITA KOMENSKEHO V BRATISLAVE No se ha especificado una descripción o un objeto social para esta compañía.

TRL 4-5

Presupuesto del proyecto 143K€

Fecha límite de participación Sin fecha límite de participación.

Descripción del proyecto Due to a high sustainability and to a straightforward tunability of the energy input (wavelength, redox potential), the use of light and electricity for the activation of organic molecules constitutes an attractive method in the toolkit of the organic chemist. Consequently, photochemistry and electrochemistry are both undergoing a renaissance in the recent decade, mainly in the form of photo- and electro- catalysis. Both of these activation modes share many traits, as they proceed via single electron transfer mechanisms. It is obvious that a method which would combine both photo- and electro- catalysis can take advantage from these similarities, while alleviating the problems encountered with application of photo- or electro- catalysis alone. Yet, combination of these two activation modes was seldom achieved so far. The objective of this action is to develop a catalytic system, which combines photochemical and electrochemical steps in order to achieve the required reduction potential for the activation of challenging substrates. The work will be initiated with a computational benchmarking study aimed at to identify the best available method for the theoretical prediction of redox potentials. This will allow for a rational design of catalytic systems, and eventually the tailoring of a set of new catalysts to specific photo-electro catalytic transformations. To achieve optimal reaction conditions, different cell designs will be tested for a photo-electrochemical test reaction. Finally, the optimized cell and the new catalysts will be applied in radical cyclizations of demanding substrates. The HI is able to provide both equipment as well as know-how in a broad variety of fields, which is imperative for such an interdisciplinary project. The project will boost the fellow’s research skills and help him to kick-start his independent research career in Slovakia.

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