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Metal EXsolved CATalysts for the CO2 valorisation to methanol: design, synthesis...

Metal EXsolved CATalysts for the CO2 valorisation to methanol: design, synthesis, and characterisation of next-generation catalysts, unravelling their structure-activity relationship The European Union goal of a 80-95% decrease of greenhouse gas emissions by 2050 requires, among other strategies, new functional materials and sustainable approaches for clean energy generation and pollutant abatement. The chemic... see more

31/10/2024

POLITO

173K€

Project Budget: 173K€

Project leader

POLITECNICO DI TORINO No se ha especificado una descripción o un objeto social para esta compañía.

TRL 4-5

PARTICIPATION DEPralty Sin fecha límite de participación.

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Financing granted El organismo HORIZON EUROPE notifico la concesión del proyecto The day 2024-10-31

HORIZON-MSCA-2021-PF-01-01: MSCA Postdoctoral Fellowships 2024 ExpectedOutcome:

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Este proyecto no cuenta con búsquedas de partenariado abiertas en este momento.

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2 Participantes

POLITO

172.75K€ | Leader

IMPERIAL COLLEGE OF SCIENCE...

N.D. | participant

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Project duration: 27 months Date Start: 2022-07-14
End date: 2024-10-31

Project leader

POLITECNICO DI TORINO No se ha especificado una descripción o un objeto social para esta compañía.

TRL 4-5

Project Budget 173K€

participation deadline Sin fecha límite de participación.

Project description The European Union goal of a 80-95% decrease of greenhouse gas emissions by 2050 requires, among other strategies, new functional materials and sustainable approaches for clean energy generation and pollutant abatement. The chemical valorisation of CO2 is a highly promising green solution involving the recycling and reuse of CO2 effluents as carbon source for fuels and chemicals, such as methanol. The low CO2 conversion, triggered by catalytic nanoparticles (NPs) deactivation by sintering and limited selectivity, however, limits its industrial growth. The first aim of this proposal is to design next-generation stable and selective catalysts for the CO2 hydrogenation to methanol, that can rival state-of-the-art materials through the ambitious achievement of 10% methanol yield. This will be done by NP exsolution, a novel route to achieve stable anchored NPs, which has barely been explored for this application, despite the superior catalytic properties unique to exsolved systems. To then unravel the lack of fundamental understanding in the catalytic mechanisms of exsolved systems, we will characterise the correlation of their structure with their reactivity and selectivity via a unique in situ/operando approach (second aim). The role of active sites such as exsolved NPs and structural defects will be elucidated by in situ/operando Infrared (FTIR) and Raman studies; we will monitor the composition and strain evolution of the materials surfaces during catalytic processing by state-of-the-art in situ photoelectron spectroscopy (XPS) and transmission electron microscopy (TEM). The unique expertise of the host supervisor in CO2 hydrogenation catalysts testing and characterisation by in situ/operando FTIR and Raman, and of the secondment group in XPS studies of catalysts on-stream, coupled with my experience in exsolved systems design and in situ TEM characterisation will advance the fields of exsolution and CO2 valorisation catalysis, allowing me to gain a unique skillset.

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