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Development of novel strategies for alkyl organoboron preparation via boryl radi...

Development of novel strategies for alkyl organoboron preparation via boryl radical reactivity Borylated molecules are some integral tools routinely used to aid molecular construction in both academia and industry. Their use in the Nobel Prize-winning Brown oxidation and Suzuki-Miyaura cross-coupling as well as Chan-Lam ami... ver más

02/06/2026

RWTH AACHEN

174K€

Presupuesto del proyecto: 174K€

Líder del proyecto

RHEINISCHWESTFAELISCHE TECHNISCHE HOCHSCHULE... No se ha especificado una descripción o un objeto social para esta compañía.

TRL 4-5

Financiación concedida El organismo HORIZON EUROPE notifico la concesión del proyecto el día 2024-04-04

Línea de financiación objetivo El proyecto se financió a través de la siguiente ayuda:

HORIZON-MSCA-2023-PF-01-01: MSCA Postdoctoral Fellowships 2023

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RWTH AACHEN

173.85K€ | Lider

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Últimas noticias

29-11-2024: IDAE En las últimas 48 horas el Organismo IDAE ha otorgado 4 concesiones

29-11-2024: ECE En las últimas 48 horas el Organismo ECE ha otorgado 2 concesiones

29-11-2024: CMVAMADRID En las últimas 48 horas el Organismo CMVAMADRID ha otorgado 37 concesiones

Duración del proyecto: 25 meses Fecha Inicio: 2024-04-04
Fecha Fin: 2026-06-02

Presupuesto del proyecto 174K€

Descripción del proyecto Borylated molecules are some integral tools routinely used to aid molecular construction in both academia and industry. Their use in the Nobel Prize-winning Brown oxidation and Suzuki-Miyaura cross-coupling as well as Chan-Lam amination make them ubiquitous in organic synthesis. The invention of methods to form C–B bonds at sp3 carbons is of strategic importance to facilitate the preparation of saturated, hence 3D, molecules. As the pharmaceutical sector is aware of the greater clinical success of 3D molecules, developing methods able to prepare these materials is a topic of continuous scientific endeavour. Central to this quest is designing synthetic strategies able to deliver, in a divergent manner, building blocks that are stable and can be used in modular cross-coupling diversifications. This project seeks to substantially expand the fields of photoredox catalysis and boron chemistry by introducing a novel class of boryl radical precursors that will enable the generation and the use of these underdeveloped species in mainstream catalysis. This strategy will constitute a divergent platform for the generation of many novel 3D borylated molecules that will then be engaged in modular cross-coupling reactivity. Importantly, this project will provide access to materials that cannot be prepared by any other method. This research capitalizes on recent developments of the Leonori group that has experience in the generation and use of boryl radicals in synthesis. The completion of such an innovative and ambitious project at RWTH Aachen University will be facilitated by generating, transferring, sharing and disseminating knowledge, and will enhance my future career following the training plan envisioned.

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